Temperature- and field-driven spin reorientations in triple-layer ruthenate SrRuO.

Title Temperature- and field-driven spin reorientations in triple-layer ruthenate SrRuO.
Authors M. Zhu; P.G. Li; Y. Wang; H.B. Cao; W. Tian; H.D. Zhang; B.D. Phelan; Z.Q. Mao; X. Ke
Journal Sci Rep
DOI 10.1038/s41598-018-22247-3
Abstract

SrRuO, the n?=?3 member of the Ruddlesden-Popper type ruthenate SrRu O, is known to exhibit a peculiar metamagnetic transition in an in-plane magnetic field. However, the nature of both the temperature- and field-dependent phase transitions remains as a topic of debate. Here, we have investigated the magnetic transitions of SrRuO via single-crystal neutron diffraction measurements. At zero field, we find that the system undergoes a ferromagnetic transition with both in-plane and out-of-plane magnetic components at T???100?K. Below T??=?50?K, the magnetic moments incline continuously toward the out-of-plane direction. At T?=?1.5?K, where the spins are nearly aligned along the c axis, a spin reorientation occurs above a critical field B, giving rise to a spin component perpendicular to the plane defined by the field direction and the c axis. We suggest that both the temperature- and field-driven spin reorientations are associated with a change in the magnetocrystalline anisotropy, which is strongly coupled to the lattice degrees of freedom. This study elucidates the long-standing puzzles on the zero-field magnetic orders of SrRuO and provides new insights into the nature of the field-induced metamagnetic transition.

Citation M. Zhu; P.G. Li; Y. Wang; H.B. Cao; W. Tian; H.D. Zhang; B.D. Phelan; Z.Q. Mao; X. Ke.Temperature- and field-driven spin reorientations in triple-layer ruthenate SrRuO.. Sci Rep. 2018;8(1):3914. doi:10.1038/s41598-018-22247-3

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